分类: 光学 >> 量子光学 提交时间: 2023-02-19
摘要: Strong coupling exhibits unique ability to preserve quantum sates between light and matter, which is essential for the development of quantum information technology. To explore the physical mechanism behind this phenomenon, we employ the tight-binding method for expanding the temporal coupled-mode theory, with the absorption spectrum formula of coupled system directly obtained in an analytical way. It reveals all the physical meaning of parameters defined in our theory, and shows how to tailor lineshapes of the coupled systems. Here, we set an example to manipulate the strong coupling in a hybrid structure composed of excitons in monolayer WS$_2$ and quasi-bound states in the continuum supported by the TiO$_2$ nanodisk metasurfaces. The simulated results show that a clear spectral splitting appeared in the absorption curve, which can be controlled by adjusting the asymmetric parameter of the nanodisk metasurfaces and well fitted through our theoretical predictions. Our work not only gives a more comprehensive understanding of such coupled systems, but also offers a promising strategy in controlling the strong light-matter coupling to meet diversified application requests.
分类: 光学 >> 量子光学 提交时间: 2023-02-19
摘要: We investigate the strong coupling between the excitons and quasi-bound states in the continuum (BIC) resonance in a bulk WS$_2$ metasurface. Here we employ the bulk WS$_2$ to construct an ultrathin nanodisk metasurface, supporting the symmetry-protected magnetic dipole (MD) quasi-BIC resonance, which can self-hybridize with the excitons and lead to a strong light-matter interaction enhancement within the structure without the necessity for an external cavity. This strong coupling can be charactered by the considerable Rabi splitting of 159 meV and the clearly anti-crossing behavior appeared in the absorption spectrum. Furthermore, we analyze such light-matter coupling by constructing a Hamiltonian model including the surplus excitons, and tune the interaction from weak coupling to strong coupling regimes via the tunability radiation loss of the quasi-BIC resonance. Our results have great potential for manipulating the exciton-polaritons at room temperature, and provide a promising prospect for photonic devices that exploit strong coupling in applications.
分类: 光学 >> 量子光学 提交时间: 2023-02-19
摘要: The emerging all-dielectric platform exhibits high-quality ($Q$) resonances governed by the physics of bound states in the continuum (BIC) that drives highly efficient nonlinear optical processes. Here we demonstrate the robust enhancement of third-(THG) and fifth-harmonic generation (FHG) from all-dielectric metasurfaces composed of four silicon nanodisks. Through the symmetry breaking, the genuine BIC transforms into the high-$Q$ quasi-BIC resonance with tight field confinement for record high THG efficiency of $3.9\times10^{-4}$ W$^{-2}$ and FHG efficiency of $4.8\times10^{-10}$ W$^{-4}$ using a moderate pump intensity of 1 GW/cm$^{2}$. Moreover, the quasi-BIC and the resonantly enhanced harmonics exhibit polarization-insensitive characteristics due to the special $C_{4}$ arrangement of meta-atoms. Our results suggest the way for smart design of efficient and robust nonlinear nanophotonic devices.
分类: 光学 >> 量子光学 提交时间: 2023-02-19
摘要: We present nonlinear optical four-wave mixing in a silicon nanodisk dimer metasurface. Under the oblique incident plane waves, the designed metasurface exhibits a multi-resonant feature with simultaneous excitations of three quasi-bound states in the continuum (BIC). Through employing these quasi-BICs with maximizing electric field energy at the input bump wavelengths, significant enhancement of third-order nonlinear processes including third-harmonic generation, degenerate and non-degenerate four-wave mixing are demonstrated, giving rise to ten new frequencies in the visible wavelengths. This work may lead to a new frontier of ultracompact optical mixer for applications in optical circuitry, ultrasensitive sensing, and quantum nanophotonics.
分类: 光学 >> 量子光学 提交时间: 2023-02-19
摘要: Tailoring optical nonlinear effects (e.g. harmonic generation, sum-frequency mixing, etc.) in the recently emerging all-dielectric platform is important for both the fundamental science and industrial development of high-efficiency, ultrafast, and miniaturized photonic devices. In this work, we propose a novel paradigm for dynamically switchable high-harmonic generation in Silicon nanodimer metasurfaces by exploiting polarization-controlled dual bound states in the continuum (BIC). Owing to the high-quality factor of BIC resonances, efficient harmonic signals including the third-harmonic generation and fifth-harmonic generation from a direct process as well as a cascaded process by degenerate four-wave mixing are obtained. Moreover, the BICs and their resonantly enhanced harmonics can be switched on or off with high selectivity respect to the fundamental pump polarization. Compared with previous reports, our work provide a simple but effective tuning strategy by fully exploring the structural symmetry and polarization degree of freedom rather than resorting to additional external stimuli, which would have great advantages in smart designing tunable and switchable nonlinear light source for chip-scale applications.